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• W2118777777 abstract "Maximum differences in the chemical free energy between a crystalline oxide and its fully amorphous counterpart at are estimated from melting point and enthalpy of fusion data for oxides in ten different metal systems (Be, Zn, Cu, Al, Cr, Fe, Ni, Zr, Sn, and Ti). The results are used to determine the relative thermodynamic stability of crystalline and amorphous phases in aqueous solutions in order to understand the possible influence of amorphism on precursor pitting sites in passive films. Variations in the degree of amorphism are treated by using different values, where , and examining the resulting effects on pH-dependent oxide solubility and equilibria. Estimated surface energies of high-angle grain boundaries are used to show that grain boundaries in crystalline oxide films may be treated as amorphous regions." @default.
• W2118777777 created "2016-06-24" @default.
• W2118777777 creator A5028936003 @default.
• W2118777777 date "2005-01-01" @default.
• W2118777777 modified "2023-09-26" @default.
• W2118777777 title "Thermodynamic Evaluation of the Effects of Amorphism on Film Breakdown and Pitting Initiation" @default.
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• W2118777777 doi "https://doi.org/10.1149/1.2048169" @default.
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