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- W2118863295 abstract "Three-chromophore systems with light-harvesting behavior were prepared, which are based on periodic mesoporous organosilica (PMO) with crystal-like ordered structure. The organic bridges of biphenyl-PMO in the pore walls act as donors and two types of dye are incorporated in the one-dimensional channels. Consecutive two-step-Förster resonance energy transfer is observed from the biphenyl moieties to mediators (diethyl-aminocoumarin or aminoacridone), followed by energy transfer from mediators to acceptors (dibenzothiacarbocyanine, indodicarbocyanine, sulforhodamine G). High energy-transfer efficiencies ranging from 70 to 80 % are obtained for two-step-FRET, indicating that the mesochannel structure with one-dimensional ordering provides spatial arrangement of chromophore pairs for an efficient direct energy transfer. The emission wavelength can be tuned by a choice of acceptor dye: 477 nm (diethylaminocoumarin), 519 nm (aminoacridone), 567 nm (sulforhodamine G), 630 nm (dibenzothiacarbocyanine), and 692 nm (indodicarbocyanine)." @default.
- W2118863295 created "2016-06-24" @default.
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- W2118863295 creator A5089057154 @default.
- W2118863295 date "2014-10-28" @default.
- W2118863295 modified "2023-09-30" @default.
- W2118863295 title "Light-Harvesting Three-Chromophore Systems Based on Biphenyl-Bridged Periodic Mesoporous Organosilica" @default.
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- W2118863295 doi "https://doi.org/10.1002/chem.201403393" @default.
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