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- W2118917785 abstract "The long-timescale behavior of adsorbed carbon monoxide on the surface of amorphous water ice is studied under dense cloud conditions by means of off-lattice, on-the-fly, kinetic Monte Carlo simulations. It is found that the CO mobility is strongly influenced by the morphology of the ice substrate. Nanopores on the surface provide strong binding sites, which can effectively immobilize the adsorbates at low coverage. As the coverage increases, these strong binding sites are gradually occupied leaving a number of admolecules with the ability to diffuse over the surface. Binding energies and the energy barrier for diffusion are extracted for various coverages. Additionally, the mobility of CO is determined from isothermal desorption experiments. Reasonable agreement on the diffusivity of CO is found with the simulations. Analysis of the 2152 cm−1 polar CO band supports the computational findings that the pores in the water ice provide the strongest binding sites and dominate diffusion at low temperatures." @default.
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- W2118917785 date "2013-12-30" @default.
- W2118917785 modified "2023-10-17" @default.
- W2118917785 title "DYNAMICS OF CO IN AMORPHOUS WATER-ICE ENVIRONMENTS" @default.
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- W2118917785 doi "https://doi.org/10.1088/0004-637x/781/1/16" @default.
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