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• W2119420820 endingPage "1546" @default.
• W2119420820 startingPage "1524" @default.
• W2119420820 abstract "Palladacyclic compounds [Pd(C6H4(C6H5CO)CNR)(NN)] [X] (R = Et, iPr, 2,6-iPr2C6H3; NN = bpy = 2,2′-bipyridine, or 1,4-(o,o′-dialkylaryl)-1,4-diazabuta-1,3-dienes; [X]− = [BF4]− or [PF6]−) were synthesized from the dimers [{Pd(C6H4(C6H5CO)CNR)(μ-Cl)}2] and NN ligands. Their interionic structure in CD2Cl2 was determined by means of 19F,1H-HOESY experiments and compared with that in the solid state derived from X-ray single-crystal studies. [Pd(C6H4(C6H5CO)CNR)(NN)] [X] complexes were found to copolymerize CO and p-methylstyrene affording syndiotactic or isotactic copolymers when bpy or 1,4-(o,o′-dimethylaryl)-1,4-diazabuta-1,3-dienes were used, respectively. The reactions with CO and p-methylstyrene of the bpy derivatives were investigated. Two intermediates derived from a single and a double insertion of CO into the PdC bonds were isolated and completely characterized in solution." @default.
• W2119420820 created "2016-06-24" @default.
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• W2119420820 date "2006-08-01" @default.
• W2119420820 modified "2023-09-25" @default.
• W2119420820 title "Synthesis, Interionic Structure, and Reactivity toward CO andp-Methylstyrene of Palladacyclic Compounds Bearingα-Diimine Ligands" @default.
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• W2119420820 doi "https://doi.org/10.1002/hlca.200690155" @default.
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