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• W2119424580 abstract "We study the interplay between hysteresis and equilibrium behavior in capillary condensation of fluids in mesoporous disordered materials via a mean-field density functional theory of a disordered lattice-gas model. The approach reproduces all major features observed experimentally. We show that the simple van der Waals picture of metastability fails due to the appearance of a complex free-energy landscape with a large number of metastable states. In particular, hysteresis can occur both with and without an underlying equilibrium transition, thermodynamic consistency is not satisfied along the hysteresis loop, and out-of-equilibrium phase transitions are possible." @default.
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• W2119424580 date "2001-07-11" @default.
• W2119424580 modified "2023-10-18" @default.
• W2119424580 title "Capillary Condensation in Disordered Porous Materials: Hysteresis versus Equilibrium Behavior" @default.
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• W2119424580 doi "https://doi.org/10.1103/physrevlett.87.055701" @default.
• W2119424580 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/11497783" @default.
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