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• W2122690037 abstract "Abstract La 2 Sn 2 O 7 and La 2 Zr 2 O 7 , two pyrochlore compounds with different B‐site cations, were prepared and used as supports for Ni in methane steam reforming. Compared with Ni/γ‐Al 2 O 3 , both Ni/La 2 Zr 2 O 7 and Ni/La 2 Sn 2 O 7 show very stable reaction performance. Whereas Ni/La 2 Zr 2 O 7 also displays reasonably high activity for the reaction, the activity of Ni/La 2 Sn 2 O 7 is extremely low. It was found that severe coking occurred with Ni/γ‐Al 2 O 3 , but no coke formation was observed on the two pyrochlore catalysts. On the reduced and spent Ni/La 2 Sn 2 O 7 catalyst, the Ni 3 Sn 2 and Ni 3 Sn alloys were detected; these alloys suppressed coke formation but also decreased the activity of the catalyst. In comparison, a large amount of La 2 O 2 CO 3 was formed on the used Ni/La 2 Zr 2 O 7 catalyst; these species reacted with the carbon deposits formed on the Ni particles and continuously restored the Ni sites. Thus, coking was effectively suppressed and the initial high activity of the catalyst was maintained. Thus, Ni/La 2 Zr 2 O 7 is a superior catalyst having the potential for industrial use." @default.
• W2122690037 created "2016-06-24" @default.
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• W2122690037 date "2014-10-30" @default.
• W2122690037 modified "2023-10-18" @default.
• W2122690037 title "Nickel-Supported on La₂Sn₂O₇and La₂Zr₂O₇Pyrochlores for Methane Steam Reforming: Insight into the Difference between Tin and Zirconium in the B Site of the Compound" @default.
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• W2122690037 doi "https://doi.org/10.1002/cctc.201402551" @default.
• W2122690037 hasPublicationYear "2014" @default.
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