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- W2122825739 abstract "The Eu(III)/(II) reaction was studied by conventional and by Type I and Type II kalousek polarography in a number of media. Reduction waves appear to fall into two groups depending upon whether inner or outer sphere complexes are formed between Eu(III) and the anion of the supporting electrolyte. The reversibility as evidenced by K-I and K-II curves increases in order of supporting electrolytes as ClO4−<Cl−<NO3−<Br−<I−<SCN− and appears to correlate only with decreasing charge at the electrode surface due to increased specific adsorption of the anions. The double anodic wave observed at low ionic strength in perchlorate is consistent with previous studies of the system and appears to have its origin in double layer effects rather than in an intermediate in the reduction. The utility of Type I and II Kalousek polarography in the study of irreversible processes is demonstrated." @default.
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- W2122825739 date "1970-05-01" @default.
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- W2122825739 title "Electrochemical studies of the EU(III)/(II) reaction by conventional and kalousek polarography" @default.
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