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• W2123282437 endingPage "3592" @default.
• W2123282437 startingPage "3592" @default.
• W2123282437 abstract "The hydrothermal synthesis, X-ray crystal structures and thermal and magnetic properties of a layered coordination polymer, [Ni(3.9)Mn(1.1)(μ(3)-OH)(2)(L(I))(2)(H(2)O)(10)]·2H(2)O (1) (L(I) = 1e,2a,4a,5e-cyclohexanetetracarboxylate), and a porous 3D coordination polymer, [Ni(4)(μ(2)-OH)(2)(μ(6)-H(2)L(IV))(2)(pymc)(4,4'-bpy)(H(2)O)(2)](OH)·9H(2)O (2) (pymc = 2-pyrimidinecarboxylate, 4,4'-bpy = 4,4'-bipyridine, L(IV) = 1e,2e,4e,5e-cyclohexanetetracarboxylate), are reported in this paper. The structure of 1 has packed separated layers, each layer being formed of M(3)(μ(3)-OH)(2) chains bridged by M(L(I))(2)via hydrogen bonds. The magnetic properties are characterized by Néel transitions to fully compensated antiferromagnets at 2.9 K and show that 1 is a metamagnet resulting from the ferrimagnetic M(3)(μ(3)-OH)(2) chains and other two metal atoms. Complex 2 is a 3D microporous coordination framework with 2D channels. The conformation of the 1,2,4,5-cyclohexanetetracarboxylate ligands (H(4)L) of complex 2 changes from L(I) (e,a,a,e) to L(IV) (e,e,e,e). The magnetic measurement indicates spin-canted antiferromagnetic behaviour, and the adsorption measurements show that 2 can selectively adsorb CO(2) gas over N(2) gas." @default.
• W2123282437 created "2016-06-24" @default.
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• W2123282437 date "2011-01-01" @default.
• W2123282437 modified "2023-10-13" @default.
• W2123282437 title "Two new 1,2,4,5-cyclohexanetetracarboxylate-bridged frameworks with metal hydroxide subunits. Synthesis, structures, magnetism and adsorption" @default.
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• W2123282437 doi "https://doi.org/10.1039/c0dt01497d" @default.
• W2123282437 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21373675" @default.
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