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• W2123311207 startingPage "83" @default.
• W2123311207 abstract "Abstract Two centuries ago solvated electrons were discovered in liquid ammonia and a century later the concept of the solvent cage was introduced. Here, we report a real time study of the dynamics of size‐selected clusters, n =20 to 60, of electrons in ammonia, and, for comparison, that of electrons in water cages. Unlike the water case, the observed dynamics for ammonia indicates the formation, through a 100 fs temperature jump, of a solvent collective motion in a 500 fs relaxation process. The agreement of the experimental results—obtained for a well‐defined n , gated electron kinetic energy, and time delay—with molecular dynamics theory suggests the critical and different role of the kinetic energy and the librational motions involved in solvation." @default.
• W2123311207 created "2016-06-24" @default.
• W2123311207 creator A5057482213 @default.
• W2123311207 creator A5073809869 @default.
• W2123311207 creator A5077807260 @default.
• W2123311207 date "2008-01-04" @default.
• W2123311207 modified "2023-10-18" @default.
• W2123311207 title "Dynamics of Electrons in Ammonia Cages: The Discovery System of Solvation" @default.
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• W2123311207 doi "https://doi.org/10.1002/cphc.200700562" @default.
• W2123311207 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18038379" @default.
• W2123311207 hasPublicationYear "2008" @default.
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