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- W2124132011 abstract "Abstract Novel diiron complexes with an Fe 2 (μ‐OMe) 2 core were studied as models of the active site of nonheme iron‐containing enzymes. X‐ray crystal structures of the complexes showed the existence of two types of ligand folding—parallel and twisted—both of which have four virtually equivalent phenolato groups sticking out from the Fe 2 O 2 rhombic plane. Cyclic voltammetry measurements revealed two or more distinct redox waves in a region of relatively high potential, in addition to known Fe II /Fe III redox waves in a region of lower potential. These new peaks were assigned to the high‐valence state of iron atoms, that is, Fe III Fe IV and Fe IV Fe IV , resonating with the phenoxyl radical(s). The split width of the redox waves ranged from 0.14 to 0.20 eV, which may be a measure of the electronic interaction of the phenolate groups through the Fe 2 (μ‐OMe) 2 core." @default.
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- W2124132011 date "2004-09-13" @default.
- W2124132011 modified "2023-10-10" @default.
- W2124132011 title "Structural and Electrochemical Studies of Novel Bis(?-methoxo)diiron complexes: Observation of FeIIIFeIV and FeIVFeIV States Resonating with Phenoxyl Radicals" @default.
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- W2124132011 doi "https://doi.org/10.1002/chem.200400114" @default.
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