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• W2125896474 abstract "Molecular simulation techniques have been utilised to investigate the effect of cross-linker type on the structural and dynamical properties of a temperature-sensitive hydrogel, poly (N-isopropyl acrylamide) (PNIPAM) across its lower critical solution temperature (LCST). PNIPAM exhibits an LCST at ∼305 K, above which it collapses and below which it is swollen. Molecular dynamics simulations of PNIPAM hydrogel cross-linked with N, N′-methylene bisacrylamide (BIS) and ethylene glycol dimethacrylate (EGD) cross-linkers were carried out below, at and above its LCST (namely 300, 305 and 310 K, respectively). Structural analysis indicates that the cross-linkers did not affect the temperature of the onset of the LCST, but did affect the degree of swelling and pore size distribution, where the EGD-cross-linked hydrogel exhibited a greater degree of structural change than that of the BIS-cross-linked hydrogel. We believe that this could be attributed to the longer chain length and more flexible nature of the EGD cross-linker compared to the BIS cross-linkers." @default.
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• W2125896474 date "2011-09-01" @default.
• W2125896474 modified "2023-10-14" @default.
• W2125896474 title "Molecular simulation study of the effect of cross-linker on the properties of poly(<i>N</i>-isopropyl acrylamide) hydrogel" @default.
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• W2125896474 doi "https://doi.org/10.1080/08927022.2011.566608" @default.
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