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- W2126078165 abstract "The absorption and laser-induced fluorescence spectra of the C̃1B2–X̃1A1 band of SO2 were simultaneously measured between 221.5 and 208 nm under jet-cooled conditions. The fluorescence quantum yields above the dissociation threshold showed irregularity, reflecting a level specificity in the predissociation rate. The vibronic-level dependence in the predissociation rate was interpreted in terms of the nodal structure of the vibrational wavefunctions, constructed from a least-squares analysis of the observed vibrational energies in the C̃ state. The vibrational wavefunctions can be categorized into two types of localized wavefunctions: one stretching along the dissociation coordinate which tends to afford a much faster dissociation rate than the other which folds perpendicularly to the dissociation coordinate." @default.
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- W2126078165 date "1998-09-01" @default.
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- W2126078165 title "Vibrational propensity in the predissociation rate of SO2( ) by two types of nodal patterns in vibrational wavefunctions" @default.
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- W2126078165 doi "https://doi.org/10.1016/s0009-2614(98)00922-1" @default.
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