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• W2127266735 abstract "Detailed interpretation of the far infrared spectra of the pyridine–I2 complex (in ternary mixtures with an inert solvent) has been attempted using models for elucidation of intermolecular dynamics between components of a liquid mixture. For the complex very diluted in an inert solvent, in the framework of the Robertson–Yarwood model, it is found that the bandshape of the υI-I mode originates from the phase relaxation of the I–I oscillator due to its anharmonic ‘indirect’ coupling with the υD-I mode. The frequency shifts and widths of the two bands observed at higher concentrations of pyridine in the mixture are then explored by applying the vibrational relaxation formalism of Kubo with the analytical expression of Fukuda, T., Ikawa, S., and Kimura, M., (1989, Chem. Phys., 133,137) to treat the ‘direct’ coupling of the transition dipole of the complex with the dipole moment of the solvent molecule. Both phase and energy relaxation contributions have been considered. It has been found that band intensities..." @default.
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• W2127266735 date "1997-10-01" @default.
• W2127266735 modified "2023-09-24" @default.
• W2127266735 title "Vibrational spectroscopic studies of the chemical dynamics in charge transfer complexes of the type iodine-pyridine 2. Intermolecular dynamics from far infrared bands" @default.
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• W2127266735 doi "https://doi.org/10.1080/002689797170473" @default.
• W2127266735 hasPublicationYear "1997" @default.
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