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• W2127783146 abstract "Poly[(S)-3-vinyl-2,2′-dihydroxy-1,1′-binaphthyl] (L*) was obtained by taking off the protecting groups of poly[(S)-3-vinyl-2,2′-bis(methoxymethoxy)-1,1′-binaphthyl] (poly-1). L* was proved to keep a stable helical conformation in solution. The application of helical L* in the asymmetric addition of diethylzinc to aldehydes has been studied. The catalytic system employing 10 mol% of L* and 150 mol% of Ti(OiPr)4 was found to promote the addition of diethylzinc to a wide range of aromatic aldehydes, giving up to 99% enantiomeric excess (ee) and up to 93% yield of the corresponding secondary alcohol at 0°C. The chiral polymer can be easily recovered and reused without loss of catalytic activity as well as enantioselectivity." @default.
• W2127783146 created "2016-06-24" @default.
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• W2127783146 date "2015-02-03" @default.
• W2127783146 modified "2023-10-14" @default.
• W2127783146 title "Optically Active Helical Poly[(<i>S</i>)-3-vinyl-2,2′-dihydroxy-1,1′-binaphthyl]: New Ligand for Asymmetric Addition of Diethylzinc to Aryl Aldehyde" @default.
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• W2127783146 doi "https://doi.org/10.1002/cjoc.201400819" @default.
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