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- W2128900144 abstract "We present a combined experimental and theoretical study of molecular methanethiol $({text{CH}}_{3}text{SH})$ adsorption on the reconstructed Au(111) surface in the temperature range between 90 and 300 K in UHV. We find that the simplest thiol molecules form two stable self-assembled monolayer (SAM) structures that are created by distinct processes. Below 120 K, a solid rectangular phase, preserving the herringbone reconstruction, emerges from individual chains of spontaneously formed dimers. At higher adsorption temperatures below 170 K, a close-packed phase forms via dissociative ${text{CH}}_{3}text{SH}$ adsorption and the formation of Au adatoms that are not incorporated into the SAM. We show that the combination of a strong substrate-mediated interaction with nondissociative dimerization and temperature activated removal of the Au(111) reconstruction drives the large-scale assembly of molecular ${text{CH}}_{3}text{SH}$ into two distinct phases." @default.
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- W2128900144 date "2009-08-03" @default.
- W2128900144 modified "2023-10-16" @default.
- W2128900144 title "Self-assembly of methanethiol on the reconstructed Au(111) surface" @default.
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- W2128900144 doi "https://doi.org/10.1103/physrevb.80.081401" @default.
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