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• W2129136783 endingPage "1657" @default.
• W2129136783 startingPage "1652" @default.
• W2129136783 abstract "Thiol-responsive symmetric triblock copolymers having single disulfide linkages in the middle blocks (called mono-cleavable block copolymers, ss-ABP(2)) were synthesized by atom transfer radical polymerization in the presence of a disulfide-labeled difunctional Br-initiator. These brush-like triblock copolymers consist of a hydrophobic polyacrylate block having pendent oligo(propylene oxide) and a hydrophilic polymethacrylate block having pendent oligo(ethylene oxide). Gel permeation chromatography and (1)H NMR results confirmed the synthesis of well-defined mono-cleavable block copolymers and revealed that polymerizations were well controlled. Because of amphiphilic nature, these copolymers self-assembled to form colloidally stable micelles above critical micellar concentration of 0.032 mg · mL(-1). In response to reductive reactions, disulfides in thiol-responsive micelles were cleaved. Atomic force microscopy and dynamic light scattering analysis suggested that the cleavage of disulfides caused dissociation of micelles to smaller-sized assembled structures in water. Moreover, in a biomedical perspective, the mono-cleavable block copolymer micelles are not cytotoxic and thus biocompatible." @default.
• W2129136783 created "2016-06-24" @default.
• W2129136783 creator A5035301452 @default.
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• W2129136783 creator A5063728387 @default.
• W2129136783 date "2011-08-19" @default.
• W2129136783 modified "2023-10-10" @default.
• W2129136783 title "New Thiol-Responsive Mono-Cleavable Block Copolymer Micelles Labeled with Single Disulfides" @default.
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• W2129136783 doi "https://doi.org/10.1002/marc.201100372" @default.
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