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- W2129202327 abstract "A series of hybrid supramolecular star polymers (SSPs) consisting of a polyoxometalate EuW10O369− (EuW10) core and different length of polystyrene arms have been fabricated by a “core-first” method, in which the anionic EuW10 clusters were firstly encapsulated by cationic molecules with trithioester terminal groups and subsequently polystyrene arms were grafted by reversible addition–fragmentation chain-transfer (RAFT) polymerization. The SSPs exhibit structurally dependent self-assembly behaviours in solution, at the air–water interface and solid state. It was found that the SSPs with short arms form large assemblies with a diameter over 100 nm in chloroform, while those with long arms tend to be mono-dispersed. Meanwhile, the distance between the EuW10 cores of adjacent SSPs in Langmuir monolayers and casting films can be precisely adjusted by PS arms, which leads to a tunable colour purity of EuW10 luminescence. This tight structure–property relationship enables the polyoxometalate-cored SSPs to act as potential building blocks for the construction of hybrid polymer materials with controllable functions." @default.
- W2129202327 created "2016-06-24" @default.
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- W2129202327 date "2014-01-01" @default.
- W2129202327 modified "2023-10-16" @default.
- W2129202327 title "Structurally dependent self-assembly and luminescence of polyoxometalate-cored supramolecular star polymers" @default.
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- W2129202327 doi "https://doi.org/10.1039/c3py01349a" @default.
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