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- W2129790106 abstract "The first total synthesis of gelsemoxonine (1) has been accomplished. Divinylcyclopropane–cycloheptadiene rearrangement of the highly functionalized substrate was successfully applied to assemble the spiro-quaternary carbon center connected to the bicyclic seven-membered core structure. A one-pot isomerization reaction of the α,β-unsaturated aldehyde to the saturated ester via the TMSCN–DBU reagent combination allowed a facile diastereoselective introduction of the latent nitrogen functionality of the unique azetidine moiety." @default.
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- W2129790106 date "2011-10-13" @default.
- W2129790106 modified "2023-10-18" @default.
- W2129790106 title "Total Synthesis of Gelsemoxonine" @default.
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- W2129790106 doi "https://doi.org/10.1021/ja208617c" @default.
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