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- W2130013406 abstract "Hyper-Rayleigh scattering experiments and quantum chemical calculations are combined to investigate the second-order nonlinear optical responses of a series of three-arm merocyanine derivatives. They exhibit an octupolar hyperpolarizability response with lower amplitude than crystal violet due to a lower extent of the photoinduced charge transfer and reduced bond length alternation. Strong effects on the second-order optical response measured close to the two-photon absorption level are clearly evidenced; for example, the effective measured polarization ratio deviates below the ideal octupolar value of 3/2 even at very low excitation power. These effects are attributed to two-photon absorption resonance, which we believe modifies dynamically the population of the ground state versus that of the excited state." @default.
- W2130013406 created "2016-06-24" @default.
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- W2130013406 date "2014-06-20" @default.
- W2130013406 modified "2023-10-16" @default.
- W2130013406 title "Experimental and Theoretical Investigation of the First-Order Hyperpolarizability of Octupolar Merocyanine Dyes" @default.
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- W2130013406 doi "https://doi.org/10.1002/cphc.201402083" @default.
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