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- W2130122088 abstract "Abstract A detailed mechanistic model has been developed to describe the methane oxidative coupling network over Li/MgO catalysts. The mechanism assumes that methane and other hydrocarbon species react directly from the gas phase with surface active oxygen centres (Eley- Rideal representation). The surface network comprises parallel and sequential elementary steps describing the following chemical processes: 1] hydrocarbon dehydrogenation, 2] non-selective partial oxidation of hydrocarbon species, 3] catalyst dehydration, 4] gaseous oxygen adsorption and active centre regeneration, 5] catalyst poisoning by carbon oxides, and 6] carbon monoxide oxidation. The surface kinetic parameters were estimated on the basis of scaling arguments and published experimental data. The surface network is combined with a homogeneous methane oxidation mechanism thus resulting in a detailed kinetic model which can account for the observed conversion levels and hydrocarbon product distributions." @default.
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- W2130122088 date "1992-03-01" @default.
- W2130122088 modified "2023-09-27" @default.
- W2130122088 title "A mechanistic kinetic model for oxidative coupling of methane over Li/MgO catalysts" @default.
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- W2130122088 doi "https://doi.org/10.1016/0920-5861(92)80161-f" @default.
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