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- W2130407104 abstract "The use of a laccase-mediator system is one of the promising possibilities for an environmentally benign pulp-bleaching process. Thus a better understanding of the mechanism for the oxidation of lignin by a laccase-mediator system would facilitate the commercialization of such a system for pulp bleaching. By using 1-hydroxybenzotriazole (1-HBT) as a mediator, it was found to be partly regenerated during the oxidation of a lignin dimer, 1-(3,4-dimethoxyphenyl)-2-(2-methoxy-phenoxy)propan-1,3-dio (I). A free radical of 1-HBT, generated by laccase, was probably responsible for the oxidation of I. The free radical of 1-HBT was, however, transformed to benzotriazole, which could not mediate the oxidation of 1. The hypothesis that 1-HBT acted as an activator or a co-substrate for laccase was not confirmed. Active oxygen species such as hydroxyl free radical (HO . ) and superoxide (O 2 .- ) were also found not to be involved in the oxidation of I." @default.
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- W2130407104 date "1998-06-01" @default.
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- W2130407104 title "Mechanistic studies of the oxidation of a non-phenolic lignin model compound by the laccase/1-hydroxybenzotriazole redox system" @default.
- W2130407104 doi "https://doi.org/10.1111/j.1470-8744.1998.tb00500.x" @default.
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