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• W2130711044 abstract "Abstract We use doubly resonant, infrared‐visible sum‐frequency generation spectroscopy (DR‐SFG) to probe vibrational and electronic properties of C 60 and K‐doped C 60 monolayers adsorbed on Ag(111) single crystal under ultra‐high vacuum (UHV). We recorded the interface SFG spectra for five visible wavelengths. We observe a strong dependence of the SFG intensity of the totally symmetric A g (2) mode of the fullerene while scanning the visible wavelength, due to the DR‐SFG phenomenon. The SFG intensity of the A g (2) mode is the strongest at 488 nm and at 532 nm for the pure and fully doped monolayers, respectively. These results demonstrate the occurrence of electron–phonon couplings at the C 60 /Ag(111) and saturated K/C 60 /Ag(111) interfaces. They enable us to determine the energy of the coupled electronic transition and to link the electronic resonance to the h u (HOMO) to t 1g (LUMO + 1) transition of C 60 ." @default.
• W2130711044 created "2016-06-24" @default.
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• W2130711044 date "2010-07-19" @default.
• W2130711044 modified "2023-10-09" @default.
• W2130711044 title "<i>In situ</i> nonlinear optical spectroscopy of electron-phonon couplings at alkali-doped C₆₀ /Ag(111) interfaces" @default.
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• W2130711044 doi "https://doi.org/10.1002/pssb.200983947" @default.
• W2130711044 hasPublicationYear "2010" @default.
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