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- W2131121812 abstract "A treatment of the theory of radiationless processes in molecules is given using the Jortner- Stepanov model. This model can be solved exactly, showing the precise conditions under which the “statistical” limit is valid. It appears that irreversibility occurs only when one deals with an exact continuum, but otherwise oscillations in the time dependence remain. In this case a radiationless transition can only occur when collisions with other molecules are present within the period of oscillation (recurrence time). Then a detailed presentation of the time dependence of two states, which can be excited and are connected with one another by a quasi-continuum, is given." @default.
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- W2131121812 date "1972-11-01" @default.
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- W2131121812 title "Analysis of the Jortner-Stepanov theory of radiationless transitions in organic molecules" @default.
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- W2131121812 doi "https://doi.org/10.1016/0031-8914(72)90151-6" @default.
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