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• W2131856988 startingPage "247" @default.
• W2131856988 abstract "Abstract The electroreduction mechanism of diheptylviologen (V 2+ ) across a self‐assembled dioleoylphosphatidylcholine (DOPC) monolayer supported on a mercury electrode has been investigated in aqueous 0.1 M KCl by the chronocoulometric technique. V 2+ is reduced in two consecutive charge steps, 2V 2+ + 3e → V + 2 and V + 2 + e → 2V 0 , involving 3/2 and 1/2 of a faraday per mole of reactant, respectively. Both charge steps are controlled by the rate of the elementary coupling step V + + V 0 → V + 2 . V 2+ acts as an electron transfer mediator from ferric and ferricyanide ions dissolved in the aqueous solution to the mercury surface across the DOPC monolayer, which is impermeable to these metal ions in the absence of V 2+ . The electron transfer mediation is more effective along the first charge step, 2V 2+ + 3e → V + 2 , and increases with the V 2+ concentration in the lipid monolayer less than proportionally, thus pointing to the radical cation V + as the most effective electron carrier from the mercury surface to the metal ions." @default.
• W2131856988 created "2016-06-24" @default.
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• W2131856988 date "1997-01-01" @default.
• W2131856988 modified "2023-10-18" @default.
• W2131856988 title "Electroreduction of Diheptylviologen in a Self-Assembled Phospholipid Monolayer on Mercury and its Role as an Electron Transfer Mediator" @default.
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• W2131856988 doi "https://doi.org/10.1002/ijch.199700029" @default.
• W2131856988 hasPublicationYear "1997" @default.
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