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- W2132237811 abstract "Abstract Metal‐oxide nanostructure‐decorated extrinsic semiconductor interfaces modified through in situ nitridation greatly expand the range of sensor interface response. Select metal‐oxide sites, deposited to an n‐type nanopore‐coated microporous interface, direct a dominant electron‐transduction process for reversible chemical sensing, which minimizes chemical‐bond formation. The oxides are modified to decrease their Lewis acidity through a weak interaction to form metal oxynitride sites. Conductometric and X‐ray photoelectron spectroscopy measurements demonstrate that in situ treatment changes the reversible interaction with the analytes NH 3 and NO. The sensor range is extended, which creates a distinct new family of responses determined by the Lewis acidity/basicity of a given analyte relative to that of the nanostructures chosen to decorate the interface. The analyte response, broadened in a substantial and predictable way by nitridation, is explained by the recently developing inverse hard/soft acid/base model (IHSAB) of reversible electron transduction." @default.
- W2132237811 created "2016-06-24" @default.
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- W2132237811 date "2014-05-26" @default.
- W2132237811 modified "2023-10-12" @default.
- W2132237811 title "Direct In Situ Nitridation of Nanostructured Metal Oxide Deposited Semiconductor Interfaces: Tuning the Response of Reversibly Interacting Sensor Sites" @default.
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- W2132237811 doi "https://doi.org/10.1002/cphc.201402108" @default.
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