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• W2132859464 endingPage "A1617" @default.
• W2132859464 startingPage "A1611" @default.
• W2132859464 abstract "There is considerable interest in developing solid electrolytes for rechargeable lithium batteries as they have the potential to increase both energy density due to incorporation of a lithium metal anode and safety of batteries due to the fact that they are nonflammable. Block copolymers with a mechanically hard non-conducting block and a soft ion-conducting block provide an avenue for obtaining highly conducting rigid solids. In this study we add surface-modified TiO2 nanoparticles to a mixture of polystyrene-block-poly(ethylene oxide) and bis(trifluoromethane)sulfonimide lithium salt. The presence of BF4− moieties on the surface of the particles was essential for obtaining macroscopically homogeneous electrolytes; macrophase separation was observed with the same nanoparticles with surfaces covered with oleic acid. The stability of these composite electrolytes against lithium metal electrodes was tested in symmetric lithium-composite electrolyte-lithium cells. The surprising result was that electrolytes with 24 wt% nanoparticles exhibited optimum stability; the amount of charge passed before dendrite formation observed in the optimized composite electrolyte was a factor of 4.7 larger than that of the neat block copolymer electrolyte. Both tensile and shear moduli of the electrolytes were non-monotonic functions of particle concentration with peaks in the vicinity of 17 to 20 wt%." @default.
• W2132859464 created "2016-06-24" @default.
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• W2132859464 date "2013-01-01" @default.
• W2132859464 modified "2023-10-08" @default.
• W2132859464 title "Nanocomposites of Titanium Dioxide and Polystyrene-Poly(ethylene oxide) Block Copolymer as Solid-State Electrolytes for Lithium Metal Batteries" @default.
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• W2132859464 doi "https://doi.org/10.1149/2.117309jes" @default.
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