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- W2133063334 abstract "Shape–memory materials (SMMs) and actuators possess the ability to respond to external stimuli such as temperature, electricity, magnetic field, and light, and change their shapes. During the process, energy is converted into mechanical deformation which makes them attractive for various applications in biomedical devices, deployable structures, artificial muscles, microdevices, sensors, etc. Traditional SMMs and actuators rely on the properties of bulk material irrespective of their nature (e.g. polymers, metallic alloys, composite materials). Very recently, polymer-brush-based nanoscale bending actuators were reported. As a consequence of the strong interchain repulsion, the overcrowded polymer chains within the polymer brush can exert forces onto the underlying substrate and deform the substrate. However, there is no empirical evidence that bending observed on the nanoscale can be adapted for actuator applications on the macroscale. Furthermore, bending alone may not be sufficient to provide the desired macroscopic actuation; axial stretching may also be required. Herein we demonstrate the bending and stretching of a soft polymeric substrate, plasticized poly(vinyl chloride) (pPVC, thickness 400 mm, Young!s Modulus 6.89 MPa), on the macroscale by grafting a model hydrophilic polymer, poly(N,N-dimethylacrylamide) (PDMA), at high graft density on the pPVC surface. As shown in Figure 1A, when PDMA" @default.
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- W2133063334 date "2011-04-21" @default.
- W2133063334 modified "2023-10-18" @default.
- W2133063334 title "Bending and Stretching Actuation of Soft Materials through Surface-Initiated Polymerization" @default.
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- W2133063334 doi "https://doi.org/10.1002/anie.201008252" @default.
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