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• W2133412864 abstract "Abstract A novel gold‐catalyzed tandem cyclization/[1,2]‐alkyl migration process of epoxy alkynes to spiropyranones has been discovered. From this process, the construction of adjacent multiple stereocenters with a new quaternary carbon atom is achieved. The gold‐catalyzed domino process is stereospecific with respect to the migrating carbon atom. A type of unusual CC bond cleavage of epoxide systems has also been discovered, which can lead to the formation of two Z alkenes and a carbonyl functional group in one step with excellent stereoselectivity. Furthermore, this efficient domino process could be achieved in the presence of the simplest and least expensive gold catalyst [NaAuCl 4 ] ⋅ 2 H 2 O with a low catalyst loading." @default.
• W2133412864 created "2016-06-24" @default.
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• W2133412864 date "2008-05-29" @default.
• W2133412864 modified "2023-10-18" @default.
• W2133412864 title "Au-Catalyzed Tandem Cyclization/[1,2]-Alkyl Migration Reaction of Epoxy Alkynes: Synthesis of Spiropyranones" @default.
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• W2133412864 doi "https://doi.org/10.1002/chem.200800194" @default.
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