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- W2133543686 abstract "The luminescent decay of excited uranyl ion has been studied over a wide temperature range in dilute aqueous acid, concentrated HClO4, H2SO4, H3PO4, a borosilicate glass, acetone, CH3CN, CF3CO2H, CH3OH, CD3OD and a polymeric film (of cellulose acetate). In those cases where it was possible to work at temperatures as low as 77 K, it proved possible to rationalise the temperature-dependence of the rate in terms of the equation k(T)=B+A exp (–Delta;E[graphic omitted]/RT). B, which is similar for all systems studied (within a factor of 3), is taken as reflecting a combination of radiative and non-radiative processes of a physical nature. The second term is characterised by high values of ΔE≠ and (like the first) the presence of kinetic isotope effects, and is taken to refer to chemical quenching, usually by a process of rapidly reversed hydrogen–atom abstraction, but (when this is impossible) by electron-abstraction." @default.
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- W2133543686 date "1979-01-01" @default.
- W2133543686 modified "2023-09-25" @default.
- W2133543686 title "Inorganic photophysics in solution. Part 2.—Temperature activation of decay processes in the luminescence of uranyl[UO2+2] ion" @default.
- W2133543686 doi "https://doi.org/10.1039/f19797500342" @default.
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