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- W2133896672 abstract "By creating two triplet excitons from one photo-excited singlet exciton, singlet fission in organic semiconductors has drawn tremendous attention for its potential applications in boosting the efficiency of solar conversion. Here, we show that this carrier-multiplication effect can also be used to dramatically improve the nonlinear optical response in organic materials. We have observed large optical nonlinearity with a magnitude of χ(3) up to 10−9 esu in pentacene films, which is further shown to be a result of singlet fission by monitoring the temporal dynamics. The potential application of such efficient nonlinear optical response has been demonstrated with a singlet-fission-induced polarization rotation." @default.
- W2133896672 created "2016-06-24" @default.
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- W2133896672 date "2015-04-02" @default.
- W2133896672 modified "2023-10-17" @default.
- W2133896672 title "Large Optical Nonlinearity Induced by Singlet Fission in Pentacene Films" @default.
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- W2133896672 doi "https://doi.org/10.1002/anie.201501396" @default.
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