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- W2135485013 abstract "We recently found that crystallization of monodisperse hard spheres from the bulk fluid faces a much higher free-energy barrier in four than in three dimensions at equivalent supersaturation, due to the increased geometrical frustration between the simplex-based fluid order and the crystal [J. A. van Meel, D. Frenkel, and P. Charbonneau, Phys. Rev. E 79, 030201(R) (2009)]. Here, we analyze the microscopic contributions to the fluid-crystal interfacial free energy to understand how the barrier to crystallization changes with dimension. We find the barrier to grow with dimension and we identify the role of polydispersity in preventing crystal formation. The increased fluid stability allows us to study the jamming behavior in four, five, and six dimensions and to compare our observations with two recent theories [C. Song, P. Wang, and H. A. Makse, Nature (London) 453, 629 (2008); G. Parisi and F. Zamponi, Rev. Mod. Phys. (to be published)]." @default.
- W2135485013 created "2016-06-24" @default.
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- W2135485013 creator A5047047018 @default.
- W2135485013 creator A5083774969 @default.
- W2135485013 date "2009-12-08" @default.
- W2135485013 modified "2023-09-23" @default.
- W2135485013 title "Hard-sphere crystallization gets rarer with increasing dimension" @default.
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- W2135485013 doi "https://doi.org/10.1103/physreve.80.061110" @default.
- W2135485013 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/20365121" @default.
- W2135485013 hasPublicationYear "2009" @default.
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