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• W2135736705 abstract "Melting-point depression by soluble impurities is an entropy-driven phenomenon. Studying partially oxidized free sodium nanoparticles, we found an additional mechanism, which is caused by insoluble impurities. Oxidization of sodium clusters with 135--192 atoms by a single oxygen molecule causes a melting-point depression of $17ifmmodepmelsetextpmfi{}6text{ }text{ }mathrm{K}$; additional oxygen amplifies the effect. This is in contrast to the behavior of bulk sodium, where the melting point does not change upon partial oxidization. First-principles density functional theory calculations reveal the interaction between the pure and the oxidized part of the cluster to be responsible for the effect. There is more structural freedom in a liquid cluster to optimize the interface between the two parts. This stabilizes the liquid phase and causes the observed, cluster-specific melting-point depression." @default.
• W2135736705 created "2016-06-24" @default.
• W2135736705 creator A5004254737 @default.
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• W2135736705 date "2008-07-11" @default.
• W2135736705 modified "2023-09-27" @default.
• W2135736705 title "Melting-Point Depression by Insoluble Impurities: A Finite Size Effect" @default.
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• W2135736705 doi "https://doi.org/10.1103/physrevlett.101.023401" @default.
• W2135736705 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18764180" @default.
• W2135736705 hasPublicationYear "2008" @default.
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