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- W2135801394 abstract "Most knowledge on catalytic reaction mechanisms has up until now been gathered with UHV-based techniques. The extrapolation of such obtained reaction parameters to the pressure range of real application conditions is called the pressure gap. The nonlinear optical technique Second Harmonic Generation (SHG) allows studies covering the whole pressure range between UHV and application pressures. Of special importance for this purpose is the possibility to distinguish coverages of different adsorbates. In this work we show how the application of phase sensitive SHG can be used to determine coverages of different adsorbates in-situ allowing the determination of important reaction parameters. Our choice of reaction is the catalytic water formation on platinum which is already widely investigated in the literature." @default.
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- W2135801394 date "1998-04-30" @default.
- W2135801394 modified "2023-09-27" @default.
- W2135801394 title "<title>In-situ investigation of catalytic reactions with second harmonic generation</title>" @default.
- W2135801394 doi "https://doi.org/10.1117/12.307126" @default.
- W2135801394 hasPublicationYear "1998" @default.
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