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- W2137171803 abstract "Recent experimental observations of time-resolved multidimensional signals in the light-harvesting antennae Fenna-Mathews-Olson [G. S. Engel et al., Nature (London) 446, 782 (2007)] show large oscillations of exciton populations coupled to the long-lived coherences. These effects may not be reproduced by the standard Redfield theory which assumes weak coupling to a bath. A more general relaxation superoperator which holds for all system-bath coupling parameter regimes is constructed by taking into account the statistics (covariances) of Lindblad equation parameters. Simulations for a model dimer reproduce all observed strong coupling effects." @default.
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- W2137171803 date "2009-05-28" @default.
- W2137171803 modified "2023-10-16" @default.
- W2137171803 title "Lindblad equations for strongly coupled populations and coherences in photosynthetic complexes" @default.
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- W2137171803 doi "https://doi.org/10.1063/1.3142485" @default.
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