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- W2137354345 abstract "This work demonstrates a novel proof-of-concept to implement pentacene derivatives as emitters for the third generation of light-emitting electrochemical cells based on small-molecules (SM-LECs). Here, a straightforward procedure is shown to control the chromaticity of pentacene-based lighting devices by means of a photoinduced cycloaddition process of the 6,13-bis(triisopropylsilylethynyl) (TIPS)-pentacene that leads to the formation of anthracene-core dimeric species featuring a high-energy emission. Without using the procedure, SM-LECs featuring deep-red emission with Commission Internationale d'Eclairage (CIE) coordinates of x = 0.69/y = 0.31 and irradiance of 0.4 μW cm−2 are achieved. After a careful optimization of the cycloaddition process, warm white devices with CIE coordinates of x = 0.36/y = 0.38 and luminances of 10 cd m−2 are realized. Here, the mechanism of the device is explained as a host–guest system, in which the dimeric species acts as the high-energy band gap host and the low-energy bandgap TIPS-pentacene is the guest. To the best of the knowledge, this work shows the first warm white SM-LECs. Since this work is based on the archetypal TIPS-pentacene and the photoinduced cycloaddition process is well-knownfor any pentacenes, this proof-of-concept could open a new way to use these compounds for developing white lighting sources." @default.
- W2137354345 created "2016-06-24" @default.
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- W2137354345 date "2015-07-14" @default.
- W2137354345 modified "2023-09-27" @default.
- W2137354345 title "Controlling the Chromaticity of Small-Molecule Light-Emitting Electrochemical Cells Based on TIPS-Pentacene" @default.
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- W2137354345 doi "https://doi.org/10.1002/adfm.201501326" @default.
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