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• W2139675388 abstract "Herein, we analyze earlier obtained and new data about peculiarities of the H/D hydrogen exchange of small C1–n-C4 alkanes on Zn-modified high-silica zeolites ZSM-5 and BEA in comparison with the exchange for corresponding purely acidic forms of these zeolites. This allows us to identify an evident promoting effect of Zn on the activation of CH bonds of alkanes by zeolite Brønsted sites. The effect of Zn is demonstrated by observing the regioselectivity of the H/D exchange for propane and n-butane as well as by the increase in the rate and a decrease in the apparent activation energy of the exchange for all C1–n-C4 alkanes upon modification of zeolites with Zn. The influence of Zn on alkane activation has been rationalized by dissociative adsorption of alkanes on Zn oxide species inside zeolite pores, which precedes the interaction of alkane with Brønsted acid sites." @default.
• W2139675388 created "2016-06-24" @default.
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• W2139675388 date "2008-12-01" @default.
• W2139675388 modified "2023-09-24" @default.
• W2139675388 title "Significant Influence of Zn on Activation of the C-H Bonds of Small Alkanes by Brønsted Acid Sites of Zeolite" @default.
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• W2139675388 doi "https://doi.org/10.1002/cphc.200800569" @default.
• W2139675388 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18972491" @default.
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