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• W2140051253 abstract "We present extended x-ray absorption fine structure (EXAFS) data at the La ${L}_{2}$ edge in LaOCl that were recorded on the $L{ensuremath{beta}}_{1}$ fluorescence line with an analyzer energy bandwidth of $1.3phantom{rule{0.3em}{0ex}}mathrm{eV}$. We show that by taking advantage of the high-energy-resolution fluorescence detection (HERFD) it is possible to extend the energy range for ${L}_{2}$ EXAFS analysis beyond the ${L}_{1}$ edge if the sample is optically thin. The arguments presented here generally apply to fluorescence-detected absorption spectroscopy if the fluorescence lines are sufficiently separated in energy. Calculations using an atomic multiplet model show that intensity due to $2p4d$ multiple-electron excitations is reduced in HERFD spectra. The technique has the potential of considerably improving EXAFS analyses at low energies $(<10phantom{rule{0.3em}{0ex}}mathrm{keV})$ when absorption edges lie within a few hundred electron volts." @default.
• W2140051253 created "2016-06-24" @default.
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• W2140051253 date "2005-07-15" @default.
• W2140051253 modified "2023-10-16" @default.
• W2140051253 title "Range-extended EXAFS at the<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi>L</mml:mi></mml:math>edge of rare earths using high-energy-resolution fluorescence detection: A study of La in LaOCl" @default.
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• W2140051253 doi "https://doi.org/10.1103/physrevb.72.014117" @default.
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