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• W2140718126 abstract "Sterical control: Density functional calculations revealed that rhodium- catalyzed hydrogenative coupling of 1,3-diynes and vicinal dicarbonyl compounds (see scheme; cod=1,5-cyclooctadiene, OTf=trifluoromethanesulfonyl) occurs through an oxidative coupling mechanism. The oxidative coupling by 1,4-addition to the conjugated diyne via a seven-membered cyclic cumulene transition state leads to the exclusive formation of the CC bond at the terminal position of the diyne with high regio- and enantioselectivity." @default.
• W2140718126 created "2016-06-24" @default.
• W2140718126 creator A5021833788 @default.
• W2140718126 creator A5042178740 @default.
• W2140718126 creator A5042928999 @default.
• W2140718126 date "2011-03-01" @default.
• W2140718126 modified "2023-09-23" @default.
• W2140718126 title "Mechanism and Origins of Regio- and Enantioselectivities in RhI-Catalyzed Hydrogenative Couplings of 1,3-Diynes and Activated Carbonyl Partners: Intervention of a Cumulene Intermediate" @default.
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• W2140718126 doi "https://doi.org/10.1002/chem.201002741" @default.
• W2140718126 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/3159924" @default.
• W2140718126 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21365696" @default.
• W2140718126 hasPublicationYear "2011" @default.
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