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- W2141304800 abstract "Abstract The solubility of ThO 2 (cr) was studied since many years but a large discrepancy in solubility values is noticed in the literature. The present work suggests that this discrepancy is related to differences in the surface properties of thorium oxide. To understand the role of surface properties on solubility values, we conducted experiments with ThO 2 (cr) spheres with reproducable surface properties. Batch dissolution experiments were conducted in 0.01 M NaCl solution at pH=3.0 and 4.0 for periods of time up to 270 days. The solutions were spiked with 229 Th to determine precipitation (sorption) rates of thorium, while dissolution rates were determined by measuring 232 Th released from ThO 2 (cr) spheres. We assume that 229 Th atoms are exchanged only with active sites involved in Th-dissolution. Using 229 Th as local sensor of attachement and detachment processes at the ThO 2 (cr) surface under close-to-equilibrium conditions, allows to assess surface reactivity of the solid during solubility experiments." @default.
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- W2141304800 date "2008-11-01" @default.
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- W2141304800 title "Discrepancies in thorium oxide solubility values: a new experimental approach to improve understanding of oxide surface at solid/solution interface" @default.
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- W2141304800 doi "https://doi.org/10.1524/ract.2008.1531" @default.
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