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• W2142155010 abstract "Solvated electrons (e−s) which are generated at the disk of a rotating ring-disk electrode (RRDE) can be oxidized at the ring electrode; the electrons were generated at different electrode materials in a 0.3 M Li salt + hexamethylphosphortriamide (HMPA) solution. By means of this RRDE technique the current distribution during e−s generation at glassy carbon was investigated: a uniform current density distribution could not be obtained during e−s generation. Also passivation of different ring electrode materials in this medium was studied. During cathodic polarization at Pt, a film, probably from the electrocatalytically destroyed solvent, was formed. This film is impermeable for e−s. At glassy carbon, however, this type of passivation was not observed. The e−s diffusion coefficient in a 0.3 M LiBr + HMPA solution was calculated at different temperatures from −s transit time measurements. The activation energy of diffusion was found to be 5.9 kJ mol−1." @default.
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• W2142155010 date "1991-02-01" @default.
• W2142155010 modified "2023-10-16" @default.
• W2142155010 title "Studies of the solvated electron in Li salt + HMPA solutions using the rotating ring-disk electrode technique" @default.
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• W2142155010 doi "https://doi.org/10.1016/0022-0728(91)85461-w" @default.
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