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- W2142632017 abstract "Three neutral bis(μ-chalcogenido)diiron(III) complexes, [{(N,N'-Pipiso)Fe(μ-E)}2] (Pipiso(-) = [(DipN)2C(cis-2,6-Me2NC5H8)](-), (Dip = C6H3Pr(I)2-2,6; E = O, S or Se) have been prepared by reactions of the iron(I) dimer [{(μ-N,N'-Pipiso)Fe}2] with O2, S8 or Se∞. Treating the μ-selenido compound [{(N,N'-Pipiso)Fe(μ-Se)}2] with O2 cleanly generated its μ-oxo counterpart, [{(N,N'-Pipiso)Fe(μ-O)}2]. X-ray crystallographic analyses of the compounds showed them to possess Fe2(μ-E)2 core structures with distorted square planar (E = O) or tetrahedral (E = S or Se) iron coordination geometries. Magnetic, (57)Fe Mössbauer spectroscopic and computational studies indicate medium to strong antiferromagnetic coupling between the two high-spin Fe(III) ions in all three compounds." @default.
- W2142632017 created "2016-06-24" @default.
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- W2142632017 date "2015-01-01" @default.
- W2142632017 modified "2023-10-14" @default.
- W2142632017 title "Neutral diiron(<scp>iii</scp>) complexes with Fe<sub>2</sub>(μ-E)<sub>2</sub>(E = O, S, Se) core structures: reactivity of an iron(<scp>i</scp>) dimer towards chalcogens" @default.
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- W2142632017 doi "https://doi.org/10.1039/c4dt03081h" @default.
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