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- W2146196825 abstract "Abstract. The currently used kinetic-fractionation (KF) model of the differential incorporation of water-molecule isotopologues into vapor-grown ice omits surface processes on crystal facets that may be important in temperature reconstructions. This article introduces the surface-kinetic fractionation model, a model that includes such surface processes, and shows that differences in deposition coefficients for water isotopologues can produce isotopic fractionation coefficients that significantly differ from those of KF theory. For example, if the deposition coefficient of H218O differs by just 5% from that of ordinary water (H216O), the resulting fractionation coefficient at 20% supersaturation may deviate from the KF value by up to about ±17‰, and even more at greater supersaturation. As a result, the surface-kinetic theory may significantly change how fractionation depends on supersaturation. Moreover, the model introduces possible new temperature dependencies from the deposition coefficients. These parameters need to be constrained by new laboratory measurements." @default.
- W2146196825 created "2016-06-24" @default.
- W2146196825 creator A5017770861 @default.
- W2146196825 date "2011-11-16" @default.
- W2146196825 modified "2023-10-16" @default.
- W2146196825 title "Theory of isotopic fractionation on facetted ice crystals" @default.
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- W2146196825 doi "https://doi.org/10.5194/acp-11-11351-2011" @default.
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