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- W2146321421 abstract "Equilibria between four-, five- and six-co-ordinated substituted and unsubstituted [Ni(β-dik)(diam)]+ complexes associated with various solvents like acetonitrile, acetone, n-butanol, formamide dimethylformamide, dimethyl sulfoxide and pyridine have been investigated in nitroethane solution at 293 K. Increasing donor strength of the donor solvents (L) as well as increasing electron-withdrawing properties of the substituents at the β-diketonate (β-dik) and the diamine (diam) ligands favours the formation of six-co-ordinated species. The results are interpreted using correlations with IR, Hammett and electrochemical data, and results of semiempirical quantum-mechanical calculations carried out within an extended CNDO/2 framework, cis–trans Isomerism is proposed for [Ni(β-dik)(diam)L2]+ due to the mechanism of stepwise co-ordination." @default.
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- W2146321421 date "1994-01-01" @default.
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- W2146321421 title "Co-ordination of solvent molecules to square-planar mixed-ligand nickel(II) complexes: a thermodynamic and quantum-mechanical study" @default.
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- W2146321421 doi "https://doi.org/10.1039/dt9940001091" @default.
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