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- W2146862979 abstract "Abstract By using the properties of fluorine such as electronic effects and leaving-group ability, two types of ring-forming reactions have been achieved starting from fluoroolefins: (i) fluorinated vinyl ketones with a vinyl and/or an aryl group, which undergo fluorine-directed and/or -activated Nazarov, Friedel-Crafts, and tandem cyclizations in their combination to construct highly functionalized and fused ring systems and (ii) gem-difluoroolefins bearing a nucleophilic center on the carbon δ to the flourines undergo intramolecular substitution for the fluorine via anti-Baldwin 5-endo-trig closures leading to ring-fluorinated heterocycles. Throughout these reactions, fluorines function as an activator of the substrates and a controller over the reaction pathways." @default.
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- W2146862979 date "2000-01-01" @default.
- W2146862979 modified "2023-10-18" @default.
- W2146862979 title "Ring constructions by the use of fluorine substituent as activator and controller" @default.
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- W2146862979 doi "https://doi.org/10.1351/pac200072091685" @default.
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