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- W2146953074 abstract "Detailed time-resolved photodissociation and caging dynamics in clusters are studied using I2−(OCS)11 as a model system. We report new observations of product channel-dependent properties of nuclear coherence in the dissociated chromophore, reflecting complex dynamics of the solvent cage. The coherence feature is most pronounced in the caged two-photon channels and its relative amplitude increases with the product size. Shorter delays, on the time scale of coherent I⋯I− motion, favor larger products, allowing for incoherent control of two-photon dissociation pathways by appropriately timing the two laser pulses. As an example of such control, I2−(OCS)2 is produced most effectively by a limited set of pump–probe excitations at short delays. We emphasize generality of these results that relate to caging dynamics in any cluster ions." @default.
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- W2146953074 date "1998-04-01" @default.
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- W2146953074 title "Transient solvent dynamics and incoherent control of photodissociation pathways in I2− cluster ions" @default.
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- W2146953074 doi "https://doi.org/10.1063/1.475928" @default.
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