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• W2147378409 abstract "ABSTRACT In this study, we used click chemistry to synthesize new linear polypeptide‐ g ‐pyrene polymers from a mono‐azido‐functionalized pyrene derivative (N 3 ‐Py) and several poly(γ‐propargyl‐ l ‐glutamate) (PPLG) oligomers. Incorporating the pyrene units as side chains enhanced the α‐helical conformations of these PPLG oligomers in the solid state, as determined using Fourier transform infrared (FTIR) spectroscopy; it also increased the temperature stability of the α‐helical secondary structures of the grafted PPLG oligomers, relative to those of the pure PPLG species, as revealed through temperature‐dependent FTIR spectroscopic analyses. In addition, the thermal properties of the PPLG‐ g ‐Py polypeptides (e.g., glass transition temperatures increased by ca. 100 °C) were superior to those of pure PPLG oligomers. Mixing the PPLG‐ g ‐Py oligomers with multiwalled carbon nanotubes (MWCNTs) in dimethylformamide led to the formation of highly dispersible PPLG‐ g ‐Py/MWCNT organic/inorganic hybrid complex materials. Fluorescence emission spectra revealed significant π–π stacking between the PPLG‐ g ‐Py oligomers and the MWCNTs in these complexes. © 2013 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2014 , 52 , 321–329" @default.
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• W2147378409 date "2013-11-18" @default.
• W2147378409 modified "2023-10-06" @default.
• W2147378409 title "Polypeptide/Multiwalled carbon nanotube hybrid complexes stabilized through noncovalent bonding interactions" @default.
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• W2147378409 doi "https://doi.org/10.1002/pola.27000" @default.
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