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- W2147652362 abstract "The integral equation formulation for radiative transfer developed by Holstein has been used to investigate the transfer of resonance fluorescence in a one-dimensional model with slab geometry. The calculations of quenched and unquenched fluorescence in pulsed and steady state systems assess the usefulness of the ‘escape factor’, which is commonly employed to describe the apparent increase in the ‘effective lifetime’ of an excited state due to radiative trapping. The results indicate that the escape factor in a steady state system depends strongly on geometry, while the corresponding escape factor in a pulsed system is less dependent on geometry, but is useful only in the latter part of the fluorescence decay. The key to both of these conlusions is the behaviour of the emitter distributions. They become very asymmetrical as a function of increasing amounts of quencher and increasing optical depth. The calculations are also applied to assessing the usefulness of a resonance filter. The results show that the limits of the filter's effectiveness in removing a resonance line emitted from another slab are set by the shape of the emitter distributions, which in turn determine the shape of the resonance line entering the filter. Finally, a comparison of the calculations is made with experimental results obtained here for Lyman-α fluorescence and elsewhere for other fluorescence systems. The comparison shows qualitative agreement and gives some guidance on applying the one dimensional results to more realistic experimental situations." @default.
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- W2147652362 date "1971-08-01" @default.
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- W2147652362 title "Resonance fluorescence transfer and radiationless deactivation in systems of intermediate optical depth" @default.
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- W2147652362 doi "https://doi.org/10.1016/0022-4073(71)90092-6" @default.
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