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- W2147702425 abstract "The photochemical decomposition of dry ozone has been studied at λ = 2537 Å. The quantum yield for the photolysis of pure ozone was proportional to the pressure of ozone; the highest quantum yield recorded was 16.7 at a pressure of 5 cmHg ozone. Variation of light intensity did not markedly affect the quantum yield, and some evidence was found for a wall termination reaction. A reaction mechanism is proposed in which O( 1 D ) atoms, formed in the primary photolysis, initiate a chain propagated by energy-rich oxygen molecules. A discussion of the nature of the energy-rich molecules is presented. Addition of inert gases to the pure ozone reduces the quantum yield to a limiting value of two. This is explained in terms of the deactivation of the energy-rich oxygen molecule. In the presence of oxygen, the quantum yield tends to zero, as a result of the reverse reaction O + O 2 + M → O 3 + M ." @default.
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- W2147702425 date "1965-10-26" @default.
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- W2147702425 title "The photolysis of ozone by ultraviolet radiation. I. The photolysis of pure, dry ozone" @default.
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- W2147702425 doi "https://doi.org/10.1098/rspa.1965.0213" @default.
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