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- W2148592992 abstract "The design and synthesis of 3D covalent organic frameworks (COFs) have been considered a challenge, and the demonstrated applications of 3D COFs have so far been limited to gas adsorption. Herein we describe the design and synthesis of two new 3D microporous base-functionalized COFs, termed BF-COF-1 and BF-COF-2, by the use of a tetrahedral alkyl amine, 1,3,5,7-tetraaminoadamantane (TAA), combined with 1,3,5-triformylbenzene (TFB) or triformylphloroglucinol (TFP). As catalysts, both BF-COFs showed remarkable conversion (96 % for BF-COF-1 and 98 % for BF-COF-2), high size selectivity, and good recyclability in base-catalyzed Knoevenagel condensation reactions. This study suggests that porous functionalized 3D COFs could be a promising new class of shape-selective catalysts." @default.
- W2148592992 created "2016-06-24" @default.
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- W2148592992 date "2014-02-07" @default.
- W2148592992 modified "2023-10-16" @default.
- W2148592992 title "3D Microporous Base-Functionalized Covalent Organic Frameworks for Size-Selective Catalysis" @default.
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- W2148592992 doi "https://doi.org/10.1002/anie.201310500" @default.
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