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• W2148778833 startingPage "693" @default.
• W2148778833 abstract "Mes*-substituted 2,3-dimethyl-1,4-diphosphabuta-1,3-diene, 1,2-diphenyl-3,4-diphosphinidenecyclobutene, 2,2-bis(methylsulfanyl)-1-phosphaethene, and 3,3-diphenyl-1,3-diphosphapropenes (Mes*=2,4,6-tri-tert-butylphenyl) were employed as P ligands of gold(I) complexes. The (E,E)-2,3-dimethyl-1,4-diphosphabuta-1,3-diene functioned as a P2 ligand for digold(I) complex formation with or without intramolecular Au–Au contact, which depends on the conformation of the 1,3-diphosphabuta-1,3-diene. The 1,2-diphenyl-3,4-diphosphinidenecyclobutene, which has a rigid s-cis PCCP skeleton, afforded the corresponding digold(I) complexes with a slight distortion of the planar diphosphinidenecyclobutene framework and intramolecular Au–Au contact. In the case of the 2,2-bis(methylsulfanyl)-1-phosphaethene, only the phosphorus atom coordinated to gold, and the sulfur atom showed almost no intra- or intermolecular coordination to gold. On the other hand, the 1,3-diphosphapropenes behaved as nonequivalent P2 ligands to afford the corresponding mono- and digold(I) complexes. Some phosphaalkene–gold(I) complexes showed catalytic activity for 1,6-enyne cycloisomerization without cocatalysts such as silver hexafluoroantimonate." @default.
• W2148778833 created "2016-06-24" @default.
• W2148778833 creator A5062400411 @default.
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• W2148778833 date "2006-11-20" @default.
• W2148778833 modified "2023-09-25" @default.
• W2148778833 title "Coordination Behavior of Sterically Protected Phosphaalkenes on the AuCl Moiety Leading to Catalytic 1,6-Enyne Cycloisomerization" @default.
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• W2148778833 doi "https://doi.org/10.1002/asia.200600155" @default.
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